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Post-combustion CO2 capture with chemical absorption: a state-of-the-art review

By Meihong Wang, Adekola Lawal, Peter Stephenson, J. Sidders and C. Ramshaw


Global concentration of CO2 in the atmosphere is increasing rapidly. CO2 emissions have an impact on global climate change. Effective CO2 emission abatement strategies such as Carbon Capture and Storage (CCS) are required to combat this trend. There are three major approaches for CCS: post-combustion capture, pre-combustion capture and oxyfuel process. Post-combustion capture offers some advantages as existing combustion technologies can still be used without radical changes on them. This makes post-combustion capture easier to implement as a retrofit option (to existing power plants) compared to the other two approaches. Therefore, post-combustion capture is probably the first technology that will be deployed. This paper aims to provide a state-of-the-art assessment of the research work carried out so far in post-combustion capture with chemical absorption. The technology will be introduced first, followed by required preparation of flue gas from power plants to use this technology. The important research programmes worldwide and the experimental studies based on pilot plants will be reviewed. This is followed by an overview of various studies based on modelling and simulation. Then the focus is turned to review development of different solvents and process intensification. Based on these, we try to predict challenges and potential new developments from different aspects such as new solvents, pilot plants, process heat integration (to improve efficiency), modelling and simulation, process intensification and government policy impact

Publisher: Elsevier Science B.V., Amsterdam
Year: 2011
DOI identifier: 10.1016/j.cherd.2010.11.005
OAI identifier:
Provided by: Cranfield CERES

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  1. (2002). A technical, economic, and environmental assessment of amine-based CO2 capture technology for power plant greenhouse gas control. doi
  2. (2010). Absorber intercooling in CO2 absorption by Piperazine-promoted Potassium Carbonate, doi
  3. (2009). Absorber model for CO2 capture by monoethanolamine – application to CASTOR pilot results, doi
  4. (2007). Adsorption of carbon dioxide on alkali-modified zeolite 13X adsorbents. doi
  5. (2001). Advanced technology for the capture of carbon dioxide from flue gases.
  6. (2004). An integrated modeling framework for carbon management technologies. doi
  7. (2004). Aqua ammonia process for simultaneous removal of CO2, SO2 and NOx, doi
  8. (2009). Carbon dioxide absorption and desorption in aqueous monoethanolamine solutions in a rotating packed bed, doi
  9. (2008). Carbon Dioxide Capture by Absorption with Potassium Carbonate.
  10. (2009). Carbon Dioxide Capture by blended Alkanolamines doi
  11. (2007). Carbon dioxide capture from existing coal-fired power plants,
  12. (2010). Carbon dioxide capture with concentrated, aqueous piperazine, doi
  13. (2007). Carbon dioxide recovery from post-combustion processes: Can gas permeation membranes compete with absorption? doi
  14. (2004). Chemical processing in high-gravity fields, from Re-engineering the chemical processing plant: Process Intensification, edited by Stankiewicz, A. and Moulijn doi
  15. (2009). Chilled ammonia process for CO2 capture", Energy Procedia, doi
  16. (2010). CO2 Capture using
  17. (2009). Current status of MHI’s CO2 recovery technology and optimization of CO2 recovery plant with a PC fired power plant, doi
  18. (2007). Development of post-combustion capture of CO2 within the CASTOR Integrated Project: First results from the pilot plant operation using
  19. (2009). Dynamic modeling and simulation of CO2 chemical absorption process for coal-fired power plants, doi
  20. (2010). Dynamic Modelling and Analysis of Post-Combustion CO2 Chemical Absorption Process for Coal-fired Power Plants, Fuel (accepted). doi
  21. (2009). Dynamic modelling and simulation of a CO2 absorber column for post-combustion doi
  22. (2009). Dynamic modelling to minimise the energy use for CO2 capture in power plant aqueous monoethanolamine, doi
  23. (2008). Effects of the temperature bulge in CO2 absorption from flue gas by aqueous monoethanolamine. Ind Eng Chem Res; doi
  24. (2007). Experimental validation of a rigorous absorber model for CO2 post-combustion capture, doi
  25. (2010). Firms gets Kingsnorth carbon capture design funding, (accessed in
  26. (2003). Fluor's econamine FG PlusSM technology. doi
  27. (1970). Gas-Liquid Reactions, McGraw-Hill, doi
  28. (2007). Initial evaluation of the impact of post-combustion capture of carbon dioxide on supercritical pulverised coal power plant part load performance, doi
  29. (2007). Integration of CO2 capture unit using single- and blended-amines into supercritical coal-fired power plants: Implications for emission and energy management, doi
  30. (2010). IPCC (2005), Intergovernmental Panel on Climate Change (IPCC) special report on carbon dioxide capture and storage, Cambridge University press,
  31. (2009). Kinetics of carbon dioxide absorption into mixed aqueous solutions of MDEA and MEA using a laminar jet apparatus and a numerically solved 2D absorption rate/kinetics model, doi
  32. (2003). Kinetics of the reactive absorption of carbon dioxide in high CO2-loaded, concentrated aqueous monoethanolamine solutions, doi
  33. (2003). Making deep reductions in CO2 emissions from coal-fired power plant using capture and storage of CO2. Proc Inst Mech Eng Part A doi
  34. (2007). Mass Transfer Characteristics of a High-voidage Rotating Packed Bed,
  35. (1981). Mass transfer process,
  36. (2003). Modeling of CO2 capture by aqueous monoethanolamine, doi
  37. (2009). Modelling and experimental studies on absorption of CO2 by Benfield solution in rotating packed bed, doi
  38. (2008). New feature to Aspen Plus 2006.5: Rate-based model of the CO2 capture process by MEA using Aspen Plus, (accessed in
  39. (2010). Noeres C, Kenig EY, Górak A doi
  40. On the modelling and simulation of sour gas absorption by aqueous amine solutions, doi
  41. (2002). Oxidative degradation of monoethanolamine, doi
  42. (2006). Pilot plant for CO2 capture with aqueous piperzine/potassium carbonate, GHGT-8, doi
  43. (2006). Pilot plant study of carbon dioxide capture by aqueous monoethanolamine, MSc Thesis,
  44. (2007). Post-combustion carbon capture from coal fired plants - solvent scrubbing, IEA Clean Coal Centre,
  45. (2010). Project details: CASTOR, "CO2 from Capture to Storage".
  46. (2004). Prospects for CO2 capture and storage. doi
  47. (2009). Rate-based process modelling study of CO2 capture with aqueous monoethanolamine solution, doi
  48. (2001). Reactive absorption: Optimal process design via optimal modelling, doi
  49. (2001). Research Needs for CO2 Capture from Flue Gas by Aqueous Absorption/Stripping, (accessed in
  50. (2009). Retrofitting CO2 capture ready fossil plants with postcombustion capture. Part 1: requirements for supercritical pulverized coal plants using solvent-based flue gas scrubbing, doi
  51. (2005). Secondment to the International Test Centre for CO2 Capture (ITC),
  52. (2007). Selection and pilot plant tests of new absorbents for post- combustion carbon dioxide capture. doi
  53. (2007). Studies of SO2- and O2- induced degradation of aqueous MEA during CO2 capture from power plant flue gas streams. doi
  54. (2004). Test results from a CO2 extraction pilot plant at Boundary Dam Coal-fired power station, doi
  55. The capture of carbon dioxide from fossil fuel fired power stations.
  56. (2010). The Press and Journal doi
  57. (2009). Thermal degradation of monoethanolamine at stripper conditions, doi
  58. (2010). Thermodynamics of aqueous potassium carbonate, piperazine, and carbon dioxide, doi
  59. (2009). Tjellander G.(2010), Maintaining a neutral water balance in a 450MWe NGCC-CCS power system with post-combustion carbon dioxide capture aimed at offshore operation. doi
  60. (2010). United Nations Environment Program, Introduction to climate change, (accessed in
  61. (2007). World energy outlook doi

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