Location of Repository

Changes in monoterpene mixing ratios during summer storms in rural New Hampshire (USA)

By K. B. Haase, C. Jordan, E. Mentis, L. Cottrell, H. R. Mayne, R. Talbot and B. C. Sive

Abstract

Monoterpenes are an important class of biogenic hydrocarbons that influence ambient air quality and are a principle source of secondary organic aerosol (SOA). Emitted from vegetation, monoterpenes are a product of photosynthesis and act as a response to a variety of environmental factors. Most parameterizations of monoterpene emissions are based on clear weather models that do not take into account episodic conditions that can drastically change production and release rates into the atmosphere. Here, the monoterpene dataset from the rural Thompson Farm measurement site in Durham, New Hampshire is examined in the context of a set of known severe storm events. While some storm systems had a negligible influence on ambient monoterpene mixing ratios, the average storm event increased mixing ratios by 0.59 ± 0.21 ppbv, a factor of 93% above pre-storm levels. In some events, mixing ratios reached the 10's of ppbv range and persisted overnight. These mixing ratios correspond to increases in the monoterpene emission rate, ranging from 120 to 1240 g km<sup>−2</sup> h<sup>−1</sup> compared to an estimated clear weather rate of 116 to 193 g km<sup>−2</sup> h<sup>−1</sup>. Considering the regularity of storm events over most forested areas, this could be an important factor to consider when modeling global monoterpene emissions and their resulting influence on the formation of organic aerosols

Topics: Environmental sciences, GE1-350, Geography. Anthropology. Recreation, G, DOAJ:Environmental Sciences, DOAJ:Earth and Environmental Sciences, Physics, QC1-999, Chemistry, QD1-999
Publisher: Copernicus Publications
Year: 2011
DOI identifier: 10.5194/acp-11-11465-2011
OAI identifier: oai:doaj.org/article:1c7ae4b23e614144af84861003fa8034
Journal:
Download PDF:
Sorry, we are unable to provide the full text but you may find it at the following location(s):
  • https://doaj.org/toc/1680-7324 (external link)
  • https://doaj.org/toc/1680-7316 (external link)
  • http://www.atmos-chem-phys.net... (external link)
  • https://doaj.org/article/1c7ae... (external link)
  • Suggested articles


    To submit an update or takedown request for this paper, please submit an Update/Correction/Removal Request.